Yea, there is a trade-off between speed and accuracy. PrintWhatYouLike aims more for accuracy- you can reformat the page exactly as you want, but its more complicated to use and takes a bit longer. Readability is fast, but you have no control over the output.
What I would really enjoy is:
1. Select the text on the page
2. Click on the bookmarklet link
3. Start to read
I wasn't able to do this quickly with PrintWhatYouLike. But maybe I am missing something.